Professional Committee of Rock and Mineral Testing Technology of the Geological Society of China, National Geological Experiment and Testing CenterHost
2019 Vol. 38, No. 6
Article Contents

Qin KUANG, Shan WU, Ting HUANG, Dai-she WU, Jing XIANG. Effect and Mechanism of Biomass Carbon and Steel Slag as Ameliorants on Soil Selenium Availability in a Typical Se-rich Area of Fengcheng City, Jiangxi Province[J]. Rock and Mineral Analysis, 2019, 38(6): 705-714. doi: 10.15898/j.cnki.11-2131/td.201901190014
Citation: Qin KUANG, Shan WU, Ting HUANG, Dai-she WU, Jing XIANG. Effect and Mechanism of Biomass Carbon and Steel Slag as Ameliorants on Soil Selenium Availability in a Typical Se-rich Area of Fengcheng City, Jiangxi Province[J]. Rock and Mineral Analysis, 2019, 38(6): 705-714. doi: 10.15898/j.cnki.11-2131/td.201901190014

Effect and Mechanism of Biomass Carbon and Steel Slag as Ameliorants on Soil Selenium Availability in a Typical Se-rich Area of Fengcheng City, Jiangxi Province

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  • BACKGROUNDThe total selenium content in the selenium-rich red soils in Fengcheng City of Jiangxi Province was relatively high, but the available selenium content directly absorbed and utilized by plants was low. The bioavailability of selenium in soils is a key factor affecting selenium in crops. OBJECTIVESTo find safe and effective ameliorants for improving the availability of selenium in selenium-rich soils. METHODSBiomass carbon and steel slag were used as modifiers, and 8 different experiments were set up. Through indoor soil test and pot experiment, the content of available selenium in the selenium-rich red soils in Fengcheng was determined by atomic fluorescence spectrometry, and the regulation effect of two kinds of ameliorants on available selenium under different treatment levels was investigated. RESULTSThe results of the soil tests showed that different amounts of biomass carbon and steel slag can increase the soil pH in the study area by 0.1-3.79 units. The results of elemental speciation analysis indicated that the ameliorant mainly controlled the soil available selenium by affecting the organically bound selenium. The soil organic matter content increased significantly after the application of biochar in the soil, but the organic matter showed a fixed effect on selenium. The available selenium content decreased by 8.4%-15.1%, resulted in the overall lower available selenium content in soils. The significant effect of steel slag on soil pH was beneficial to the activation of selenium in soils, and the soil available selenium content can be increased by 1.4 to 2.0 times. The results of the pot experiment showed that the selenium content of Chinese cabbage increased by more than 30% after treatment with steel slag, while the selenium content of Chinese cabbage decreased by 7.14%-42.8% after treatment with biochar. CONCLUSIONSThis study shows that biochar is not suitable for regulating the availability of selenium in the soil of the study area. Steel slag can be used as a control material for soil selenium availability in the study area, which not only realizes solid waste recycling, but also improves the availability of selenium in soil.
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  • [1] 李杰, 刘久臣, 汤奇峰, 等.川西高原地区水体中硒含量及分布特征研究[J].岩矿测试, 2018, 37(2):183-192.

    Google Scholar

    Li J, Liu J C, Tang Q F, et al.Study of the content and distribution of selenium in water samples from the Western Sichuan Plateau and the incidence of Kaschin Beck disease[J].Rock and Mineral Analysis, 2018, 37(2):183-192.

    Google Scholar

    [2] 王锐, 余涛, 杨忠芳, 等.富硒土壤硒生物有效性及影响因素研究[J].长江流域资源与环境, 2018, 27(7):1647-1654.

    Google Scholar

    Wang R, Yu T, Yang Z F, et al.Bioavailability of soil selenium and its influencing factors in selenium-enriched soil[J].Resources and Environment in the Yangtze Basin, 2018, 27(7):1647-1654.

    Google Scholar

    [3] 曹容浩.福建省龙海市表层土壤硒含量及影响因素研究[J].岩矿测试, 2017, 36(3):282-288.

    Google Scholar

    Cao R H.Study on selenium content of surface soils in Longhai, Fujian and its influencing factors[J].Rock and Mineral Analysis, 2017, 36(3):282-288.

    Google Scholar

    [4] 杨琼, 侯青叶, 顾秋蓓, 等.广西武鸣县典型土壤剖面Se的地球化学特征及其影响因素研究[J].现代地质, 2016, 30(2):455-462. doi: 10.3969/j.issn.1000-8527.2016.02.022

    CrossRef Google Scholar

    Yang Q, Hou Q Y, Gu Q B, et al.Study of geochemical characteristics and influencing factors of soil selenium[J].Geoscience, 2016, 30(2):455-462. doi: 10.3969/j.issn.1000-8527.2016.02.022

    CrossRef Google Scholar

    [5] Rayman M P, Sargent M, Infante H G.Food-chain selenium and human health:Emphasis on intake[J].The British Journal of Nutrition, 2008, 100(2).DOI:10.1017/S0007114508922522.

    CrossRef Google Scholar

    [6] 郭文慧, 刘庆, 史衍玺, 等.施硒对紫甘薯硒素累积及产量和品质的影响研究[J].中国粮油学报, 2016, 31(9):31-37. doi: 10.3969/j.issn.1003-0174.2016.09.006

    CrossRef Google Scholar

    Guo W H, Liu Q, Shi Y X, et al.Effects of applying selenium on the accumulation of selenium, yield, and quality of purple sweetpotato[J].Journal of the Chinese Cereals and Oils Association, 2016, 31(9):31-37. doi: 10.3969/j.issn.1003-0174.2016.09.006

    CrossRef Google Scholar

    [7] 穆婷婷, 杜慧玲, 景小兰, 等.外源硒对谷子产量因子及硒含量的影响[J].作物杂志, 2017, 14(1):73-78.

    Google Scholar

    Mu T T, Du H L, Jing X L, et al.Effects of exogenous selenium on yield components and selenium content in grain of foxtail millet[J].Crops, 2017, 14(1):73-78.

    Google Scholar

    [8] 谢邦廷, 贺灵, 江官军, 等.中国南方典型富硒区土壤硒有效性调控与评价[J].岩矿测试, 2017, 36(3):273-281.

    Google Scholar

    Xie B T, He L, Jiang G J, et al.Regulation and evaluation of selenium availability in Se-rich soils in Southern China[J].Rock and Mineral Analysis, 2017, 36(3):273-281.

    Google Scholar

    [9] 谢珊妮, 宗良纲, 张琪惠, 等.3种改良剂对强酸性高硒茶园土壤硒有效性调控效果与机理[J].茶叶科学, 2017, 37(3):299-307. doi: 10.3969/j.issn.1000-369X.2017.03.010

    CrossRef Google Scholar

    Xie S N, Zong L G, Zhang Q H, et al.Effects of three amendments on selenium availability of highly acidic and Se-rich soil in tea garden and their relative mechanisms[J].Journal of Tea Science, 2017, 37(3):299-307. doi: 10.3969/j.issn.1000-369X.2017.03.010

    CrossRef Google Scholar

    [10] 廖桥, 彭博, 李碧雄.炉渣建材资源化利用现状[J].重庆建筑, 2018, 17(3):53-57. doi: 10.3969/j.issn.1671-9107.2018.03.53

    CrossRef Google Scholar

    Liao Q, Peng B, Li B X.A review of resource utilization of slag building material[J].Chongqing Architecture, 2018, 17(3):53-57. doi: 10.3969/j.issn.1671-9107.2018.03.53

    CrossRef Google Scholar

    [11] 杨慧, 刘立晶, 刘忠军, 等.我国农田化肥施用现状分析及建议[J].农机化研究, 2014, 36(9):260-264. doi: 10.3969/j.issn.1003-188X.2014.09.059

    CrossRef Google Scholar

    Yang H, Liu L J, Liu Z J, et al.Analysis and suggestions of agricultural fertilizer application in China[J].Agricultural Mechanization Research, 2014, 36(9):260-264. doi: 10.3969/j.issn.1003-188X.2014.09.059

    CrossRef Google Scholar

    [12] 王怀臣, 冯雷雨, 陈银广.废物资源化制备生物质炭及其应用的研究进展[J].化工进展, 2012, 31(4):907-914.

    Google Scholar

    Wang H C, Feng L Y, Chen Y G.Advances in biochar production from wastes and its applications[J].Chemical Industry and Engineering Progress, 2012, 31(4):907-914.

    Google Scholar

    [13] 王晨晔, 陈艳, 郭占成, 等.以钢渣为原料合成Ca-Mg-Al-Fe层状双金属氢氧化物及其对甲基橙的吸附[J].过程工程学报, 2018, 18(3):570-574.

    Google Scholar

    Wang C Y, Chen Y, Guo Z C, et al.Preparation of Ca-Mg-Al-Fe layered double hydroxides using steel-making slag as raw material and its adsorption to methyl orange[J].The Chinese Journal of Process Engineering, 2018, 18(3):570-574.

    Google Scholar

    [14] 邓腾灏博, 谷海红, 仇荣亮.钢渣施用对多金属复合污染土壤的改良效果及水稻吸收重金属的影响[J].农业环境科学学报, 2011, 30(3):455-460.

    Google Scholar

    Deng Teng H B, Gu H H, Qiu R L.Ameliorative effects of steel slag application on multi-metal contaminated soil and heavy metal uptake of rice[J].Journal of Agro-Environment Science, 2011, 30(3):455-460.

    Google Scholar

    [15] 韩笑, 周越, 吴文良, 等.富硒土壤硒含量及其与土壤理化性状的关系——以江西丰城为例[J].农业环境科学学报, 2018, 37(6):1177-1183.

    Google Scholar

    Han X, Zhou Y, Wu W L, et al.Selenium content of farmland soils and their relationship with main soil properties in Fengcheng, Jiangxi[J].Journal of Agro-Environment Science, 2018, 37(6):1177-1183.

    Google Scholar

    [16] 李家熙, 张光弟.人体硒缺乏与过剩的地球化学环境特征及其预测[M].北京:地质出版社, 2000.

    Google Scholar

    Li J X, Zhang G D.Characteristics and Prediction of Human Selenium Deficiency and Excess Geochemical Environment[M].Beijing:Geological Publishing House, 2000.

    Google Scholar

    [17] 诸旭东, 宗良纲, 马迅, 等.内源调控与外源补硒对红壤中硒有效性及水稻产量的影响[J].土壤通报, 2016, 47(2):398-404.

    Google Scholar

    Zhu X D, Zong L G, Ma X, et al.Effects of endogenous and exogenous regulation on effectiveness of selenium and rice yield in selenium enriched soil[J].Chinese Journal of Soil Science, 2016, 47(2):398-404.

    Google Scholar

    [18] 瞿建国, 徐伯兴, 龚书椿.连续浸提技术测定土壤和沉积物中硒的形态[J].环境化学, 1997, 16(3):277-283.

    Google Scholar

    Qu J G, Xu B X, Gong S C.Sequential extraction techniques for determination of selenium speciation in soils and sediments[J].Environmental Chemistry, 1997, 16(3):277-283.

    Google Scholar

    [19] 贺攀红, 杨珍, 荣耀, 等.氢化物发生-电感耦合等离子体发射光谱法测定铀矿地质样品中痕量硒[J].岩矿测试, 2016, 35(2):139-144.

    Google Scholar

    He P H, Yang Z, Rong Y, et al.Determination of trace selenium in uranium-bearing geological samples by hydride generation-inductively coupled plasma-optimal emission spectrometry[J].Rock and Mineral Analysis, 2016, 35(2):139-144.

    Google Scholar

    [20] 陈再明, 陈宝梁, 周丹丹.水稻秸秆生物碳的结构特征及其对有机污染物的吸附性能[J].环境科学学报, 2013, 33(1):9-19.

    Google Scholar

    Chen Z M, Chen B L, Zhou D D.Composition and sorption properties of rice-straw derived biochars[J].Acta Scientiae Circumstantiae, 2013, 33(1):9-19.

    Google Scholar

    [21] 赵世翔, 于小玲, 李忠徽, 等.不同温度制备的生物质炭对土壤有机碳及其组分的影响:对土壤活性有机碳的影响[J].环境科学, 2017, 38(1):333-342.

    Google Scholar

    Zhao S X, Yu X L, Li Z H, et al.Effects of biochar pyrolyzed at varying temperatures on soil organic carbon and its components:Influence on the soil active organic carbon[J].Environmental Science, 2017, 38(1):333-342.

    Google Scholar

    [22] 赵世翔, 于小玲, 李忠徽, 等.不同温度制备的生物质炭对土壤有机碳及其组分的影响:对土壤腐殖物质组成及性质的影响[J].环境科学, 2017, 38(2):769-782.

    Google Scholar

    Zhao S X, Yu X L, Li Z H, et al.Effects of biochar pyrolyzed at varying temperatures on soil organic carbon and its components:Influence on the composition and properties of humic substances[J].Environmental Science, 2017, 38(2):769-782.

    Google Scholar

    [23] Wang D, Xue M Y, Wang Y K, et al.Effects of straw amendment on selenium aging in soils mechanism and influential factors[J].Science of the Total Environment, 2019, 657(20):871-881.

    Google Scholar

    [24] 袁金华, 徐仁扣.生物质炭对酸性土壤改良作用的研究进展[J].土壤, 2012, 44(4):541-547. doi: 10.3969/j.issn.0253-9829.2012.04.003

    CrossRef Google Scholar

    Yuan J H, Xu R K.Research progress of amelioration effects of biochars on acid soils[J].Soil, 2012, 44(4):541-547. doi: 10.3969/j.issn.0253-9829.2012.04.003

    CrossRef Google Scholar

    [25] 韩学博.不同生物质炭对植烟土壤理化性状、重金属生物有效性及烤烟生长的影响[D].临安: 浙江农林大学, 2017.http://cdmd.cnki.com.cn/Article/CDMD-10341-1017273810.htm

    Google Scholar

    Han X B.Effect of Different Biochars on Soil Physical and Chemical Properties, Heavy Metal Bioavailability and Tobacco Growth[D].Lin'an: Zhejiang Agriculture & Forestry University, 2017.

    Google Scholar

    [26] 朱李俊, 刘国威, 王磊, 等.钢渣对稀土矿区酸性土壤的改良效果[J].安徽农业科学, 2016, 44(6):159-162. doi: 10.3969/j.issn.0517-6611.2016.06.054

    CrossRef Google Scholar

    Zhu L J, Liu G W, Wang L, et al.Improvement effect of steel slag on acid soil in rare earth mining area[J].Journal of Anhui Agricultural Sciences, 2016, 44(6):159-162. doi: 10.3969/j.issn.0517-6611.2016.06.054

    CrossRef Google Scholar

    [27] Kamei-Ishikawa N, Tagami K, Uchida S.Sorption kinetics of selenium on humic acid[J].Journal of Radioanalytical and Nuclear Chemistry, 2007, 274(3):555-561. doi: 10.1007/s10967-006-6951-8

    CrossRef Google Scholar

    [28] 卢再亮, 李九玉, 徐仁扣.钢渣与生物质炭配合施用对红壤酸度的改良效果[J].土壤, 2013, 45(4):722-726.

    Google Scholar

    Lu Z L, Li J Y, Xu R K.Amelioration effects of steel slag combined with biochar on red soil acidity[J].Soil, 2013, 45(4):722-726.

    Google Scholar

    [29] 花莉, 金素素, 唐志刚.生物质炭输入对土壤CO2释放影响的研究[J].安徽农业科学, 2012, 40(11):6501-6503. doi: 10.3969/j.issn.0517-6611.2012.11.061

    CrossRef Google Scholar

    Hua L, Jin S S, Tang Z G.Effect of bio-charcoal on release of carbon dioxide in soil[J].Journal of Anhui Agricultural Sciences, 2012, 40(11):6501-6503. doi: 10.3969/j.issn.0517-6611.2012.11.061

    CrossRef Google Scholar

    [30] 何振立, 杨肖娥, 祝军, 等.中国几种土壤中的有机态硒及其分布特征[J].环境科学学报, 1993, 13(3):281-287.

    Google Scholar

    He Z L, Yang X E, Zhu J, et al.Organic selenium and its distribution in soils[J].Journal of Environmental Science, 1993, 13(3):281-287.

    Google Scholar

    [31] 章海波, 骆永明, 吴龙华, 等.香港土壤研究Ⅱ.土壤硒的含量、分布及其影响因素[J].土壤学报, 2005, 42(3):404-410. doi: 10.3321/j.issn:0564-3929.2005.03.009

    CrossRef Google Scholar

    Zhang H B, Luo Y M, Wu L H, et al.Hong Kong soil researches Ⅱ.Distribution and content of selenium in soils[J].Acta Pedologica Sinica, 2005, 42(3):404-410. doi: 10.3321/j.issn:0564-3929.2005.03.009

    CrossRef Google Scholar

    [32] 王文艳, 张丽萍, 刘俏.黄土高原小流域土壤阳离子交换量分布特征及影响因子[J].水土保持学报, 2012, 26(5):123-127.

    Google Scholar

    Wang W Y, Zhang L P, Liu Q.Distribution and affecting factors of soil cation exchange capacity in watershed of the Loess Plateau[J].Journal of Soil and Water Conservation, 2012, 26(5):123-127.

    Google Scholar

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