2020 Vol. 36, No. 12
Article Contents

JIA Lei, LIU Wentao, TANG Dehao, CAI Pengjie, CUI Zhenang. DISTRIBUTION CHARACTERISTICS AND ECOLOGICAL RISK ASSESSMENT OF HEAVY METALS IN SURFACE SEDIMENTS IN SANYA BAY AND SURROUNDING WATERS[J]. Marine Geology Frontiers, 2020, 36(12): 22-31. doi: 10.16028/j.1009-2722.2020.029
Citation: JIA Lei, LIU Wentao, TANG Dehao, CAI Pengjie, CUI Zhenang. DISTRIBUTION CHARACTERISTICS AND ECOLOGICAL RISK ASSESSMENT OF HEAVY METALS IN SURFACE SEDIMENTS IN SANYA BAY AND SURROUNDING WATERS[J]. Marine Geology Frontiers, 2020, 36(12): 22-31. doi: 10.16028/j.1009-2722.2020.029

DISTRIBUTION CHARACTERISTICS AND ECOLOGICAL RISK ASSESSMENT OF HEAVY METALS IN SURFACE SEDIMENTS IN SANYA BAY AND SURROUNDING WATERS

  • Based on the chemical analysis of Cu, Zn, Pb, Cr, As, Cd and Hg in 73 surface sediment samples in Sanya Bay and surrounding waters, the distribution characteristics of heavy metals were identified, the sources and influencing factors of heavy metals were discussed, and the ecological risk assessment was carried out by various means. The results show that the average contents of Cu, Zn, Pb, Cr, As, Cd and Hg in the study area were 12.77, 60.11, 21.11, 43.84, 7.05, 0.067 and 0.022 μg/g, respectively. The area with high content of As was the north of Xi Mao Zhou, while the content distribution of other heavy metals was generally low along the coast and gradually increased toward the sea. The contents of Cr and Hg were lossed compared with the background values, while the other heavy metals were slightly enriched. The content distribution of Zn, Pb and Cr conformed to the law of “grain size control effect”, and the material source was weathering and denudation of terrigenous detritus. Cu may be influenced by human activities in addition to terrestrial erosion. Cd and Hg were mainly from coastal sewage discharge. As was mainly from sewage discharge, agricultural application, cage aquaculture, etc. The total heavy metal pollution is in the low level standard, and the potential ecological risk of total heavy metals was also low, which reflected the overall fine sediment ecological environment of the study area, and the coastal area is better than the offshore sea area. The average pollution degree of single heavy metal was ranked as Cd>Pb>Zn>As=Cu>Cr>Hg, Cd and Pb were in the medium pollution level standard, while other heavy metals were in the low pollution level standard. The average degree of potential ecological risk of single heavy metals was in the low standard, ranking as Cd>Hg>As>Pb>Cu>Cr>Zn. Cd is the heavy metal element with the highest degree of pollution and potential ecological risk in the study area, so its prevention and control should be strengthened.

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  • [1] LI X D,POON C S,LIU P S. Heavy metal contamination of urban soils and street dusts in Hong Kong[J]. Applied Geochemistry,2001,16(11-12):1361-1368. doi: 10.1016/S0883-2927(01)00045-2

    CrossRef Google Scholar

    [2] 沈芳,毛龙江,邓晓茜,等. 江苏海岸沉积物重金属空间分布与污染性评价再分析[J]. 首都师范大学学报(自然科学版),2018,39(5):62-71.

    Google Scholar

    [3] 曾维特,杨永鹏,张东强,等. 海南岛北部海湾沉积物重金属来源、分布主控因素及生态风险评价[J]. 环境科学,2018,39(3):1085-1094.

    Google Scholar

    [4] 巩慧敏,刘永,肖雅元,等. 近海海水和表层沉积物重金属污染与生态风险评价:以海南新村港为例[J]. 农业现代化研究,2018,39(4):700-708.

    Google Scholar

    [5] MUCHA A P,VASCONCELOS M T S D,BORDALO A A. Macrobenthic community in the Douro estuary:relations with trace metals and natural sediment characteristics[J]. Environmental Pollution,2003,121(2):169-180. doi: 10.1016/S0269-7491(02)00229-4

    CrossRef Google Scholar

    [6] 甘华阳,何海军,夏真,等. 海南岛洋浦湾沉积物重金属和营养元素的污染评价与来源分析[J]. 地球与环境,2018,46(5):463-474.

    Google Scholar

    [7] 方利江,葛春盈,蒋红,等. 舟山海域表层沉积物重金属分布、来源及潜在生态风险评价[J]. 海洋环境科学,2019,38(5):769-775. doi: 10.12111/j.mes20190518

    CrossRef Google Scholar

    [8] 丁喜桂,叶思源,高宗军. 近海沉积物重金属污染评价方法[J]. 海洋地质动态,2005,21(8):31-36. doi: 10.3969/j.issn.1009-2722.2005.08.009

    CrossRef Google Scholar

    [9] 贾振邦,霍文毅,赵智杰,等. 应用次生相富集系数评价柴河沉积物重金属污染[J]. 北京大学学报(自然科学版),2000,36(6):808-812.

    Google Scholar

    [10] 柴小平,魏娜,任世军,等. 杭州湾及其邻近海域表层沉积物的沉积环境分区及重金属污染特征分析[J]. 海洋科学,2019,43(8):29-35. doi: 10.11759/hykx20190212004

    CrossRef Google Scholar

    [11] ALI R J,ALIREZA R B,AMIRHOSSEIN S T,et al. Spatial distribution,ecological and health risk assessment of heavy metals in marine surface sediments and coastal seawaters of fringing coral reefs of the Persian Gulf,Iran[J]. Chemosphere,2017,185(1):1090-1111.

    Google Scholar

    [12] DAVUTLUOGLU O I,SECKIN G,ERSU C B,et al. Heavy metal content and distribution in surface sediments of the Seyhan River,Turkey[J]. Journal of Environmental Management,2011,92(9):2250-2259. doi: 10.1016/j.jenvman.2011.04.013

    CrossRef Google Scholar

    [13] 亚力士. 三亚湾近岸海域及其珊瑚生长区重金属污染现状与评价[D]. 南宁: 广西大学, 2018.

    Google Scholar

    [14] 王玉杰. 三亚湾近海沉积物重金属污染与评价[J]. 资源节约与环保,2015(9):68-69. doi: 10.3969/j.issn.1673-2251.2015.09.054

    CrossRef Google Scholar

    [15] 刘建波,刘洁,陈春华,等. 三亚湾表层沉积物中重金属污染特征及生态风险评价[J]. 环境科学与管理,2012,37(7):106-109. doi: 10.3969/j.issn.1673-1212.2012.07.028

    CrossRef Google Scholar

    [16] 海南省区域地质志编制委员会. 海南省区域地质志[R]. 海口: 海南省地质调查院, 2012.

    Google Scholar

    [17] 中国海湾志编纂委员会. 中国海湾志第十一分册(海南省海湾)[M]. 北京: 海洋出版社, 1999: 1-426.

    Google Scholar

    [18] 刘文涛, 石要红, 贾磊, 等. 三亚陆海统筹区综合地质调查报告[R]. 广州: 广州海洋地质调查局, 2018.

    Google Scholar

    [19] 三亚市生态环境局. 2018年三亚市环境状况公报[EB/OL]. [2019/06/03]. http://www.sanya.gov.cn/sthjsite/zjgbxx/201906/ad6f6e66df954514bb1ba55850c97438.shtml.

    Google Scholar

    [20] HAKANSON L. An ecological risk index for aquatic pollution control:a sedimentological approach[J]. Water Reserch,1980,14(08):975-1001. doi: 10.1016/0043-1354(80)90143-8

    CrossRef Google Scholar

    [21] 赵一阳, 鄢明才. 中国浅海沉积物地球化学[M]. 北京: 科学出版社, 1994: 1-203.

    Google Scholar

    [22] 甘华阳,梁开,郑志昌. 珠江口表层沉积物中微量元素地球化学[J]. 海洋地质与第四纪地质,2010,30(4):131-139.

    Google Scholar

    [23] KANG X M,SONG J M,YUAN H M,et al. Speciation of heavy metals in different grain sizes of Jiaozhou Bay sediments:Bioavailability,ecological risk assessment and source analysis on a centennial timescale[J]. Ecotoxicology and Environmental Safety,2017,143(1):296-306.

    Google Scholar

    [24] HAMDOUN H,VAN-VEEN E,BASSET B,et al. Characterization of harbor sediments from the English Channel:Assessment of heavy metal enrichment,biological effect and mobility[J]. Marine Pollution Bulletin,2015,90(1/2):273-280.

    Google Scholar

    [25] XU F J,HU B Q,YUAN S Q,et al. Heavy metals in surface sediments of the continental shelf of the South Yellow Sea and East China Sea:Sources,distribution and contamination[J]. Catena,2018,160(1):194-200.

    Google Scholar

    [26] MORELLI G,GASPARON M,FIERRO D,et al. Historical trends in trace metal and sediment accumulation in intertidal sediments of Moreton Bay,Southeast Queensland,Australia[J]. Chemical Geology,2012,300/301(2):152-164.

    Google Scholar

    [27] HUANG P,LI T G,LI A C,et al. Distribution,enrichment and sources of heavy metals in surface sediments of the North Yellow Sea[J]. Continental Shelf Research,2014,73(2):1-13.

    Google Scholar

    [28] CHATTERJEE M,SILVA F E,SARKAR S,et al. Distribution and possible source of trace elements in the sediment cores of a tropical macrotidal estuary and their ecotoxicological significance[J]. Environment International,2007,33:346-356. doi: 10.1016/j.envint.2006.11.013

    CrossRef Google Scholar

    [29] 何海军,甘华阳,何金先,等. 海南岛南部滨海沉积物中重金属分布特征及生态风险评价[J]. 海洋地质前沿,2017,33(3):47-55.

    Google Scholar

    [30] GIBBS R J. Metals in the sediments along the Hudson River estuary[J]. Environment International,1994,20(4):507-516. doi: 10.1016/0160-4120(94)90199-6

    CrossRef Google Scholar

    [31] 甘华阳,何海军,张卫坤,等. 三亚河沉积物中重金属生态风险评价与污染历史[J]. 生态环境学报,2015,24(11):1878-1885.

    Google Scholar

    [32] 易志全,杨艺文,张际标,等. 湛江港海水中铜、锌、铅、镉的周年变化与水质评价[J]. 广东海洋大学学报,2011,31(1):73-79. doi: 10.3969/j.issn.1673-9159.2011.01.014

    CrossRef Google Scholar

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