Citation: | LI Yao-Yao, LI Jian-Feng. 2024. Soil Heavy Metal Pollution and Health Risk Assessment in a Tin Mining Area. South China Geology, 40(4): 712-724. doi: 10.3969/j.issn.2097-0013.2024.04.010 |
To evaluate the impact of mining activities on heavy metal pollution and health risks in the soil of a mining area, this paper systematically studied a tin mining area with a relatively simple geological background using the ground accumulation index method and Monte Carlo health risk assessment method. The results showed that: (1) The average heavy metal content in the soil of the study area was ranked in descending order: As>Zn>Pb>Cu>Ni>Cr>Cd>Hg. Only the average value of As exceeded the screening value (GB 15618—2018), while the average values of the other seven heavy metal elements did not exceed the standard; (2) Among them, the relatively high concentration areas of Cu, Pb, Zn, Cd, As, and Cr are located near the mining area and altered (mineralized) granite; (3) The land accumulation index method reveals that the pollution of As in the soil of the study area is relatively prominent, with higher levels of Pb and Cd pollution, lower levels of Cu, Zn, and Ni pollution, and almost no pollution of Cr and Hg; (4) Correlation analysis and principal component analysis indicate that the sources of heavy metal elements in soil mainly include natural sources and mining sources; (5) The health risk assessment results of Monte Carlo simulation indicate that children are more susceptible to the effects of heavy metal exposure, with As and Ni posing a higher risk of cancer for both children and adults; Sensitivity analysis further emphasizes the significant impact of As and Ni on health risks in different populations. In summary, there are slight heavy metal pollution and risk in a certain tin mining area, which are mainly controlled by the weathering of altered granite, safe and controllable.
[1] | 安文超,孙立娥,马立科,张书武.2022.某典型工业聚集区遗留地土壤重金属污染特征及健康风险评价[J]. 湖南师范大学自然科学学报,45(5):108-116. |
[2] | 曾晓娜. 2022. 湖南省某铅锌冶炼区土壤重金属空间分布特征与剖面分析[D]. 南华大学硕士学位论文. |
[3] | 常 通,何 漪,朱 莎,彭 程,王 韬,魏 滨.2024.淄博市土壤Cd和Pb的污染状况评价及健康风险评估[J]. 环境与健康杂志,41(5):399-403. |
[4] | 陈蕾洁,刘德良,谭玉勇.2023.铜死亡在肝癌中的研究进展[J]. 中南大学学报(医学版),48(9):1368-1376. |
[5] | 陈希清,秦拯纬,李剑锋,夏 杰,张遵遵,卢友月,付建明.2021.湘南骑田岭南坡环境地球化学特征研究[J]. 华南地质,37(3):298-312. doi: 10.3969/j.issn.2097-0013.2021.03.004 |
[6] | 董曼慧,夏卫生,周 浩,朱捍华.2023.湖南省地块尺度土壤重金属污染及成因研究[J]. 环境科学与技术,46(S1):60-66. |
[7] | 杜 牵. 2024. 基于风险评估和深度强化学习的自动驾驶决策方法研究[D]. 齐鲁工业大学硕士学位论文. |
[8] | 黄 卉. 2022. 湖南某矿区土壤重金属污染评价研究[D]. 中南林业科技大学硕士学位论文. |
[9] | 江诚毅. 2020. 湖南某矿区农田土壤与作物中重金属污染情况及其健康风险评价[D]. 湖南农业大学硕士学位论文. |
[10] | 蒋艳萍,彭 耀,尹宇莹,茹赛红,赵 芳,胡 芳.2024.长沙市土壤重金属污染特征及其生态与健康风险评估[J]. 中国资源综合利用,42(5):166-169. doi: 10.3969/j.issn.1008-9500.2024.05.043 |
[11] | 李剑锋,冯李霄.2023.湖南某锡矿区土壤重金属污染及健康风险评价[J]. 中国地质,50(3):897-910. doi: 10.12029/gc20220825003 |
[12] | 李剑锋,冯李霄,陈希清,付建明,卢友月,马可蒙,谢昊霖.2023.大义山东南部土壤重金属分布特征及其风险评价[J]. 环境工程技术学报,13(1):287-294. doi: 10.12153/j.issn.1674-991X.20210658 |
[13] | 刘 静,左维华,刘贞敏,于 坤,孟 琳.2024.ICP-AES测定洗涤剂中铅、镉、铬、砷、磷元素的含量[J]. 质量与认证,(8):92-95. |
[14] | 刘 越,郑志坚,李雪莹,龙奕妃,刘 洋,王 茜,孟春燕.2024.白血病患者血液和尿液中10种重金属元素测定及其相关性研究[J]. 中国煤炭工业医学杂志,27(3):280-284. |
[15] | 马 杰,佘泽蕾,王胜蓝,邓 力,刘 萍,孙 静.2023.基于蒙特卡罗模拟的煤矸山周边农用地土壤重金属健康风险评估[J]. 环境科学,44(10):5666-5678. |
[16] | 生态环境部. 2018. 土壤环境质量农用地土壤污染风险管控标准(试行):GB 15618—2018[S]. 北京:中国环境科学出版社. |
[17] | 王袆曼,葛 勤,危 超,李 翔,刘海燕,李昕妍. 南方某尾矿区地下水金属元素来源解析及健康风险评价[J/OL]. 环境科学. https://doi.org/10.13227/j.hjkx.202405145. |
[18] | 吴文伟,沈 城,沙晨燕,林匡飞,吴 健,谢雨晴,周 璇.2024.城市工业地块土壤重金属污染风险评价与源解析[J]. 生态环境学报,33(5):791-801. |
[19] | 闫 帅. 2019. 湖南湘潭地区土壤地球化学特征及健康风险评价[D]. 中国地质大学硕士学位论文. |
[20] | 杨 博,熊 健,李 伟,谢鹏程,杨崛园,黄瑞卿,吕学斌. 2024. 基于蒙特卡罗模拟的拉萨城区土壤重金属健康风险评价[J]. 环境化学,43(4):1339-1352. |
[21] | 游 萍,彭 达,李 灿,曹 慧.2024.湖南某锡矿尾矿库周边土壤重金属污染特征及其来源分析[J]. 湖南有色金属,40(3):87-92. doi: 10.3969/j.issn.1003-5540.2024.03.021 |
[22] | 喻宁华,佘佳荣,段俊敏,郑 琼,李梓铭,黄 丽,范友华.2022.湖南毛竹笋及产地土壤重金属与健康风险研究[J]. 西北林学院学报,37(4):166-172. |
[23] | 张菊琴,李东东,胡 珂,崔晓垒,张亚萍,安婷婷.2024.污染土壤生物修复技术研究进展[J]. 化工矿产地质,46(3):224-229. |
[24] | 张 煜,胡俊良,刘劲松,陈华清,杨 雪,赵震乾,刘芳枝.2018.湖南香花岭某钨矿区土壤中重金属的污染特征及生态风险研究[J]. 安全与环境工程,25(3):117-124. |
[25] | 郑立龙,张德程,郝连成,代友旭,张健康,李先锋,任开文,刘 建,孔凡全,王勇峰.2024. 广东雷州东部土壤重金属分布特征、来源分析及健康风险评价[J/OL]. 中国地质. http://kns.cnki.net/kcms/detail/11.1167.P.20240618.1339.002.html. |
[26] | Borgonovo E, Plischke E. 2016. Sensitivity analysis: A review of recent advances[J]. European Journal of Operational Research, 248(3): 869-887. doi: 10.1016/j.ejor.2015.06.032 |
[27] | Clarkson T W, Magos L, Myers G J. 2003. The toxicology of mercury—current exposures and clinical manifestations[J]. New England Journal of Medicine, 349(18): 1731-1737. doi: 10.1056/NEJMra022471 |
[28] | Förstner U, Ahlf W, Calmano W. 1993. Sediment quality objectives and criteria development in Germany[J]. Water Science and technology, 28(8-9): 307-316. |
[29] | Helton J C, Davis F J. 2003. Latin hypercube sampling and the propagation of uncertainty in analyses of complex systems[J]. Reliability Engineering & System Safety, 81(1): 23-69. |
[30] | Hughes M F, Beck B D, Chen Y, Lewis A S, Thomas D J. 2011. Arsenic exposure and toxicology: a historical perspective[J]. Toxicological Sciences, 123(2): 305-332. doi: 10.1093/toxsci/kfr184 |
[31] | International Agency for Research on Cancer. 2012. A review of human carcinogens: personal habits and indoor combustions[M]. |
[32] | Li Z Y, Ma Z W, Van Der Kuijp T J, Yuan Z W, Huang L. 2014. A review of soil heavy metal pollution from mines in China: Pollution and health risk assessment[J]. Science of the Total Environment, 468: 843-853. |
[33] | Lu G Y, Wong D W. 2008. An adaptive inverse-distance weighting spatial interpolation technique[J]. Computers & geosciences, 34(9): 1044-1055. |
[34] | Navas-Acien A, Silbergeld E K, Pastor-Barriuso R, Guallar E. 2008. Arsenic exposure and prevalence of type 2 diabetes in US adults[J]. JAMA, 300(7): 814-822. |
[35] | Saltelli A, Ratto M, Tarantola S, Campolongo F, Commission E. 2006. Sensitivity analysis practices: Strategies for model-based inference[J]. Reliability engineering & system safety, 91(10-11): 1109-1125. |
[36] | Smith A H, Marshall G, Yuan Y, Ferreccio C, Liaw J, von Ehrenstein O, Steinmaus C, Bates M N, Selvin S. 2006. Increased mortality from lung cancer and bronchiectasis in young adults after exposure to arsenic in utero and in early childhood[J]. Environmental health perspectives, 114(8): 1293-1296. |
[37] | Tchounwou P B, Yedjou C G, Patlolla A K, Sutton, D J. 2012. Heavy metal toxicity and the environment[M]. //Luch A. (eds). Molecular, Clinical and Environmental Toxicology: Volume 3: Environmental Toxicology. |
Location (a) and sampling point map (b) of the research area
Spatial distribution of heavy metal concentration in soil of the research area
Bubble chart of soil heavy metal accumulation index in the research area
Correlation analysis chart of heavy metal elements in the study area
Probability distribution of non carcinogenic health risks
Probability distribution of carcinogenic health risks
Sensitivity analysis of non carcinogenic and carcinogenic health risks