2013 Vol. 33, No. 3
Article Contents

GAN Huayang, LIANG Kai, LIN Jinqing, ZHENG Zhichang, YAN Zhangcun. DISTRIBUTION AND ACCUMULATION OF ARSENIC, CADMIUM AND MERCURY IN COASTAL WETLAND SEDIMENT OF NORTHERN BEIBU GULF[J]. Marine Geology & Quaternary Geology, 2013, 33(3): 15-28. doi: 10.3724/SP.J.1140.2013.03015
Citation: GAN Huayang, LIANG Kai, LIN Jinqing, ZHENG Zhichang, YAN Zhangcun. DISTRIBUTION AND ACCUMULATION OF ARSENIC, CADMIUM AND MERCURY IN COASTAL WETLAND SEDIMENT OF NORTHERN BEIBU GULF[J]. Marine Geology & Quaternary Geology, 2013, 33(3): 15-28. doi: 10.3724/SP.J.1140.2013.03015

DISTRIBUTION AND ACCUMULATION OF ARSENIC, CADMIUM AND MERCURY IN COASTAL WETLAND SEDIMENT OF NORTHERN BEIBU GULF

  • The spatial distribution, accumulation mechanism and controlling factors of Arsenic, Cadmium and Mercury in the last hundred years were studied based on the chemical and 210Pb, 137Cs dating data from the surface and coring sediments retrieved from the coastal wetland of north Beibu Gulf within a water depth of 0~6 m. The surface sediment is dominated by sand. The grain size of the sediment in the eastern part is coarser than that in the western part to the Dafeng river estuary. The contents of As, Cd, Hg and organic matter in the surface sediment are 8.11±5.80 μg/g、0.08±0.11 μg/g、0.034±0.028 μg/g and (0.73±0.74)%, respectively. High anomalies are found in the top part of the Tieshangang bay, the east estuary of the Nanliu river, the Qinzhou bay and the middle part of the Dafeng river estuary. Grain size is the principle factor controlling the elements distribution pattern in the surface sediment. The average sedimentation rates are 0.93 cm/a, 1.75 cm/a and 1.35 cm/a for the three cores collected from the Qin river estuary, Nanzhou (Nanliu) river estuary and Shankou mangrove conservation area during the period from 1920s to 2008, determined by 210Pb and 137Cs dating. The contents of As, Cd and Hg show an increasing trend in the period from 1985s to 2008, particularly for the cores retrieved from the estuaries of Qin river and Nanliu river due to the impacts of human activities.
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  • [1] Doody J P. The conservation of British saltmarshes[C]//Saltmarshes:morphodynamics, conservation and engineering significance. Cambridge:Cambridge University Press, 1992:80-114.

    Google Scholar

    [2] 吴黎黎, 李树华. 广西滨海湿地生态系统的恢复与保护措施[J]. 广西科学院学报, 2010, 26(1):62-66.

    Google Scholar

    [WU Lili, LI Shuhua. The restoration and protections of coastal wetland ecosystem in Guangxi[J]. Journal of Guangxi Academy of Science, 2010, 26(1):62-66.]

    Google Scholar

    [3] 韩秋影, 黄小平, 施平等. 华南滨海湿地的退化趋势、原因及保护对策[J]. 科学通报, 2006, 52(增刊Ⅱ):102-107.[HAN Qiuying, HUANG Xiaoping, SHI Ping, et al. Degradation, reasons and protection strategy of south China costal wetland[J]. Chinese Science Bulletin, 2006

    Google Scholar

    , 52(suppl Ⅱ):102-107.]

    Google Scholar

    [4] Manahan S E. Environmental Chemistry[M]. 7th. Boca Raton, FL:Lewis Press, 2000:898.

    Google Scholar

    [5] Ennouri R, Chouba L, Magni P, et al. Spatial distribution of trace metals (Cd, Pb, Hg, Cu, Zn, Fe and Mn) and oligo-elements (Mg, Ca, Na and K) in surface sediments of the Gulf of Tunis (Northern Tunisia)[J]. Environmental Monitoring and Assessment, 2010, 163(1-4):229-239.

    Google Scholar

    [6] Li Q, Wu Z, Chu B, et al. Heavy metals in coastal wetland sediments of the Pearl River Estuary, China[J]. Environmental Pollution, 2007, 49(2):158-164.

    Google Scholar

    [7] Baptista Neto J, Gingele F, Leipe T, et al. Spatial distribution of heavy metals in surficial sediments from Guanabara Bay:Río de Janeiro, Brasil[J]. Environmental Geology, 2006, 49(7):1051-1063.

    Google Scholar

    [8] Hyun S, Lee C H, Lee T, et al. Anthropogenic contributions to heavy metal distributions in the surface sediments of Masan Bay, Korea[J]. Marine Pollution Bulletin, 2007, 54(7):1059-1068.

    Google Scholar

    [9] Chatterjee M, Massolo S, Sarkar S K, et al. An assessment of trace element contamination in intertidal sediment cores of Sunderban mangrove wetland, India for evaluating sediment quality guidelines[J]. Environmental Monitoring and Assessment, 2009, 150(1-4):307-322.

    Google Scholar

    [10] Vane C H, Harrison I, Kim A W, et al. Organic and metal contamination in surface mangrove sediments of South China[J]. Marine Pollution Bulletin, 2009, 58(1):134-144.

    Google Scholar

    [11] Janaki-Raman D, P. J M, Srinivasalu S, et al. Trace metal enrichments in core sediments in Muthupet mangroves, SE coast of India:application of acid leachable technique[J]. Environmental Pollution, 2007, 145(1):245-257.

    Google Scholar

    [12] Alvarez-Iglesias P, Quintana B, Rubio B, et al. Sedimentation rates and trace metal input history in intertidal sediments from San Simón Bay (Ría de Vigo, NW Spain) derived from 210Pb and 137Cs chronology[J]. Journal of Environmental Radioactivity, 2007, 98(3):229-250.

    Google Scholar

    [13] Andrewsa J E, Samwaysc G, Shimmield G B. Historical storage budgets of organic carbon, nutrient and contaminant elements in saltmarsh sediments:Biogeochemical context for managed realignment, Humber Estuary, UK[J]. Science of the Total Environment, 2008, 405(1-3):1-13.

    Google Scholar

    [14] Irabien M J, Cearreta A, Leorri E, et al. A 130 year record of pollution in the Suances estuary (southern Bay of Biscay):Implications for environmental management[J]. Marine Pollution Bulletin, 2008, 59(10):1719-1727.

    Google Scholar

    [15] Jara-Marini M E, Soto-Jimenez M F, Paez-Osuna F. Trace metals accumulation patterns in a mangrove lagoon ecosystem, Mazatlan Harbor, southeast Gulf of California[J]. Journal of Environmental Science and Health A, Toxic/Hazardous Substances & Environmental Engineering, 2008, 43(9):995-1005.

    Google Scholar

    [16] Díaz-Asencio M, Alonso-Hernández C, Bolanos-Alvarez Y, et al. One century sedimentary record of Hg and Pb pollution in the Sagua estuary (Cuba) derived from 210Pb and 137Cs chronology[J]. Marine Pollution Bulletin, 2009, 59(4-7):108-115.

    Google Scholar

    [17] Ruiz-Fernández A C, Frignani M, Hillaire-Marcel C, et al. Trace Metals (Cd, Cu, Hg, and Pb) Accumulation recorded in the Intertidal mudflat sediments of three coastal lagoons in the Gulf of California, Mexico[J]. Estuaries and Coasts, 2009, 32(3):551-564.

    Google Scholar

    [18] 廉雪琼, 王运芳, 陈群英. 广西近岸海域海水和沉积物及生物体中的重金属[J]. 海洋环境科学, 2001, 20(2):59-62.

    Google Scholar

    [LIAN Xueqiong, WANG Yunfang, CHEN Qunying. Assessment on heavy metals in seawater, surface sediments and organisms at Guangxi inshore[J]. Marine Environmental Science, 2001, 20(2):59-62.]

    Google Scholar

    [19] 廉雪琼. 广西近岸海域沉积物中重金属污染评价[J]. 海洋环境科学, 2002, 21(3):39-42.

    Google Scholar

    [LIAN Xueqiong. The assessment on the pollution of heavy metals in sediment of Guangxi inshore[J]. Marine Environmental Science, 2002, 21(3):39-42.]

    Google Scholar

    [20] 蓝锦毅, 廉雪琼, 巫强. 广西近岸海域沉积物环境质量现状与评价[J]. 海洋环境科学, 2006, 25(S1):57-59.

    Google Scholar

    [LAN Jinyi, LIAN Xueqiong, WU Qiang. Status and evaluation on the environmental quality of sediment in Guangxi coast[J]. Marine Environmental Science, 2006, 25(S1):57-59.]

    Google Scholar

    [21] 夏鹏, 孟宪伟, 印萍,等. 广西北海潮间带沉积物中重金属的污染状况及其潜在生态危害[J]. 海洋科学进展, 2008, 26(4):471-477.

    Google Scholar

    [XIA Peng, MENG Xianwei, YIN Ping,et al. Heavy metal pollution and its potential ecological risk in the sediments from the Beihai intertidal zone of Guangxi province[J]. Advances in Marine Science. 2008, 26(4):471-477.]

    Google Scholar

    [22] Xia P, Meng X, Feng A, et al. Geochemical characteristics of heavy metals in coastal sediments from the northern Beibu Gulf (SW China):the background levels and recent contamination[J]. Environmental Earth Science, 2011, DOI:10.1007/s12665-011-1343-y.

    Google Scholar

    [23] Xia P, Meng X, Yin P, et al. Eighty-year sedimentary record of heavy metal inputs in the intertidal sediments from the Nanliu River estuary, Beibu Gulf of South China Sea[J]. Environmental Pollution, 2011, 159(1):92-99.

    Google Scholar

    [24] 莫永杰. 北部湾北部浅海沉积物的粒度类型[J]. 热带海洋, 1990, 9(1):87-93.

    Google Scholar

    [MO Yongjie. Grain size types of sediment of the shallow waters in northern Beibu gulf[J]. Tropic Oceanology, 1990, 9(1):87-93.]

    Google Scholar

    [25] 广东省海岸带和海涂资源综合调查大队, 广东省海岸带和海涂资源综合调查领导小组办公室. 广东省海岸带和海涂资源综合调查报告[M]. 北京:海洋出版社, 1987:101-105.[The investigation team and leading group of the coastal fishery resource in Guangdong Province.The investigation report for the coastal fishery resource in Guangdong Province[M].Beijing:China Ocean Press, 1987:101

    Google Scholar

    -105.]

    Google Scholar

    [26] 莫永杰. 广西溺谷湾海岸地貌特征[J]. 海洋通报, 1990, 9(6):57-60.

    Google Scholar

    [MO Yongjie. Geomorphic features of drowned valley bays of Guangxi coast[J]. Marine Science Bulletin, 1990, 9(6):57-60.]

    Google Scholar

    [27] 张忠华, 胡刚, 梁士楚. 广西红树林资源与保护[J]. 海洋环境科学, 2007, 26(3):275-282.

    Google Scholar

    [ZHANG Zhonghua, HU Gang,LIANG Shichu. Mangrove resources and conservation in Guangxi[J]. Marine Environmental Science, 2007, 26(3):275-282.]

    Google Scholar

    [28] 张桂宏. 广西沿海地区潮汐特性分析[J]. 人民珠江, 2009(1):29-30.[ZHANG Guihong.Tide character analysis of Guangxi coastal area[J]. Pear River, 2009

    Google Scholar

    (1):29-30.]

    Google Scholar

    [29] 广西壮族自治区地质矿产局. 广西壮族自治区区域地质志[M]. 北京:地质出版社, 1985:5-475.[Bureau of Geology and Mineral Resources of Guangxi Province. Regional geology of Guangxi Province[M]. Beijing:Geological Publishing House, 1985:5

    Google Scholar

    -475.]

    Google Scholar

    [30] 黎广钊, 刘敬合, 方国祥. 南流江三角洲沉积特征及其环境演变[J]. 广西科学, 1994, 1(3):21-25.

    Google Scholar

    [LI Guangzhao, LIU Jinhe, FANG Guoxiang. Sedimentary characteristics of the Nanliu river delta and its environmental evolution[J]. Guangxi Sciences, 1994, 1(3):21-25.]

    Google Scholar

    [31] 夏威岚, 薛滨. 吉林小龙湾沉积速率的210Pb和137Cs年代学方法测定[J]. 第四纪研究, 2004, 24(1):123-125.

    Google Scholar

    [XIA Weilan, XUE Bin. 210Pb和137Cs method of chronological measurement for the sedimentation rate of Xiaolongwan, Jinlin province[J]. Quaternary Research, 2004, 24(1):123-125.]

    Google Scholar

    [32] Lu X, Matsumoto E. LEADAT:a MATLAB-based program for lead-210 data analysis of sediment cores[J]. Acta Oceanologica Sinica, 2006, 25(6):128-137.

    Google Scholar

    [33] Appleby P. Three decades of dating recent sediments by fallout radionuclides:a review[J]. The Holocene, 2008, 18(1):83-93.

    Google Scholar

    [34] Shepard F P. Nomenclature based on sand-silt-clay ratios[J]. Journal Sedimentary Petrology, 1954, 24:151-158.

    Google Scholar

    [35] 孙双文, 王毅, 兰健. 2006年夏季及冬季北部湾东部的海洋水文与环流[C]//北部湾海洋科学研究论文集. 北京:海洋出版社, 2009:64-72.[SUN Shuangwen, WANG Yi, LAN Jian. Hydrographic condition and circulation in the Beibu Gulf in water and summer of 2006[C]//Colloquium of marine science research for Beibu Gulf section I. Beijing, China Ocean Press, 2009

    Google Scholar

    :64-72.]

    Google Scholar

    [36] Weis D A, Callaway J C, Gersberg R M. Vertical accretion rates and heavy metal chronologies in wetland sediments of the Tijuana Estuary[J]. Estuary, 2001, 24(6A):840-850.

    Google Scholar

    [37] 李贞, 李珍, 张卫国,等. 广西钦州湾海岸带孢粉组合和沉积环境演变[J]. 第四纪研究, 2010, 30(3):598-608.

    Google Scholar

    [LI Zhen, LI Zhen, ZHANG Weiguo, et al. Pollen assemblage and sedimentary environment evolution in the coastal zone in Qinzhou bay, Guangxi province[J]. Quaternary Research, 2010, 30(3):598-608.]

    Google Scholar

    [38] 张乔民, 温孝胜, 宋朝景,等. 红树林潮滩沉积速率测量与研究[J]. 热带海洋, 1996, 15(4):57-62.

    Google Scholar

    [ZHANG Qiaomin, WEN Xiaosheng, SONG Chaojin, et al. The measurement and study on dedimentation rates in mangrove tidal flats[J]. Tropic Oceanology, 1996, 15(4):57-62.]

    Google Scholar

    [39] 全为民, 李春鞠, 沈盎绿,等. 崇明东滩湿地营养盐与重金属的分布与累积[J]. 生态学报, 2006(10):3324-3331.[QUAN Weimin, LI Chunju, SHEN Anglv, et al. Distribution and accumulation of nutrients and heavy metals in Dongtan wetlands on Chongming Island, China[J]. Acta Ecologica Sinica, 2006

    Google Scholar

    (10):3324-3331.]

    Google Scholar

    [40] 朱丹婷, 李铭红, 李侠. 互花米草群落对重金属元素的循环和富集特征[J]. 安徽农业科学, 2010, 38(3):1203-1205

    Google Scholar

    , 1208.[Zhu Danting, Li minhong, Li Xia. Cycle and enrichment characteristics of Spatina alterniflora community on heavy metal elements[J]. Journal of Anhui Agricultural Science, 2010, 38(3):1203-1205, 1208.]

    Google Scholar

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